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Researchers explore strategies to bury CO2 in concrete buildings

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One of the most powerful tools for mitigating the impact of climate change could be a material that is so common we tend not to think about it very much โ€“ concrete.

The worldโ€™s most widely used building material, concrete has an impact on carbon emissions โ€“ both as a burden and a benefit. The production of cement โ€“ one of the key components of concrete โ€“ produces relatively large amounts of carbon emissions, so mitigating these could make a big difference. But over its lifetime, concrete also has the ability to uptake carbon from the air.

Now, a new collaboration between a team of researchers led byย Daman Panesar, a professor in the University of Torontoโ€™s department of civil and mineral engineering in the Faculty of Applied Science & Engineering, andย theย Canada Green Building Councilย (CAGBC) will identify the potential and implications of low-carbon approaches and technologies and how they might capture large amounts of CO2 and trap it in concrete.

โ€œBurying Carbon in Buildings: Advancing Carbon Capture and Utilization in Cementitious Building Materialsโ€ is funded by a recently-announced $1.7 million contribution by the Government of Canada.

โ€œCurrently, several low-carbon concrete framework documents have been produced worldwide and most of these roadmaps have set 2050 carbon reduction targets related to several levers, such as clinker-cement ratio, alternative fuel useย and carbon capture, storage and sequestration,โ€ says Panesar.

While there has been preliminary work on several carbon utilization approaches, few have been implemented on a large scale. Panesar and her team will examine the challenges associated with scale-up of these strategiesย and explore new technologies that can effectively turn built infrastructure into a carbon sink.

โ€œNatural carbonation of concrete occurs by a chemical reaction between the constituents of concrete, particularly cement, and atmospheric carbon dioxide โ€“ and it has the potential to occur throughout the life of the concrete,โ€ says Panesar.

โ€œHowever, accelerated or enforced carbonation approaches are relatively new technologies, which can also be referred to as carbon capture and utilization technologies, and can be introduced at different life stagesย such as during manufacture or at end-of-life.โ€

Some examples of carbonation processes that will be explored and assessed include: CO2ย injection, elevated CO2ย exposure, mineral carbonation using recycled or waste CO2, industry by-products used to replace cement and subsequent CO2ย curing, as well as the potential for synthetic treated aggregates.

โ€œAll of these techniques need further understanding of the implications and potential for negative emission technologies such as carbon capture utilization approaches,โ€ Panesar says.

Another challenge for both new and existing structures is ensuring that any change to the formulations of concrete โ€“ for example, using lower-carbon components or absorbing more CO2ย during curing โ€“ doesnโ€™tย come at the expense of its required structural and material design properties, including strength and durability.

โ€œFor example, considering natural carbonation processes, the mechanism related to the potential for increased vulnerability of reinforced concrete elements to steel corrosion, concrete degradation and shortened service lives is fairly well understood.โ€ says Panesar.

โ€œFor existing infrastructure, the situation becomes more complex because there is a need to account for and interpret the role of age-related cracking on the CO2ย uptake of concrete, as well as in conjunction with other predominant degradation issues in Canada, such as freeze-thaw cycles.โ€

Finally, researchers will need to develop benchmarks and other standardized tools to accurately account for the carbon uptake in building materials.

โ€œCurrently, there is no harmonized measure of concrete carbonation and the differences in measurements and reporting add an extra dimension of complexity when trying to compare between different concrete formulations and/or CO2ย uptake technologies,โ€ says Panesar.

โ€œCarbon accounting is critical to enable us to determine the relative environmental impacts of the various approaches and to be able to estimate or forecast the impacts of deploying these new technologies in the coming decades.โ€

One of the strengths of the new collaboration is that it provides a built-in pathway for new research findings to get translated into industry, as well as into new policies and regulations.

โ€œAs the national organization representing members and stakeholders across the green building spectrum, CAGBC can access industry expertise to help advance research and mobilize the sector to implement market solutions,โ€ says Thomas Mueller, president and CEO of the Canada Green Building Council.

โ€œWe are proud to partner with the University of Toronto on a project that has the potential to significantly reduce embodied carbon emissions from the cement industry. The results will contribute to the collective effort to decarbonize construction.โ€

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